Deuteron-induced reactions on natural Zr from threshold to 50 MeV: production of Y
E. M. Martinsen · A. S. Voyles · K. C. W. Li🇿🇦 · M. S. Basunia · L. A. Bernstein · H. L. O. Ekeberg · M. Hussain🇵🇰 · J. T. Morrell · S. M. Qaim · S. Siem🇳🇴 · M. S. Uddin · H. Zaneb
Two stacks of thin Zr foils were irradiated with 30 and 50 MeV deuterons, respectively, using the Lawrence Berkeley National Laboratory -Inch Cyclotron, to investigate this production pathway for the promising PET tracer Y. Nineteen excitation functions for Zr(,) reactions were measured over a beam energy range of -- MeV, where the independent cross sections for Zr(,)Nb and Zr(,)Y were measured for the first time. The well-characterized Fe(,)Co, Ni(,)Co, Ni(,)Co, Ni(,)Cu, Ti(,)Sc and Ti(,)V monitor reactions were used to determine the deuteron beam current throughout the stacks. All cross sections were determined using High Purity Germanium (HPGe) detector -ray spectroscopy. A variance minimization technique was employed to simultaneously constrain the deuteron beam currents with multiple monitor reactions, thus reducing systematic uncertainties. An additional channels are reported for reactions on the nickel, titanium, and iron monitor foils, leading to a total of excitation functions, with reaction channels reported for the first time in this work. The measured excitation functions are compared to calculations provided by the reaction modeling codes , , and , as well as the data library. The degree of agreement between theory and experiments is discussed. The physical yields for Zr(,)Y and other yttrium isotopes produced are calculated and compared to other production pathways.