Photo-Induced Quenching of the 229Th Isomer in a Solid-State Host
J. E. S. Terhune🇺🇸 · R. Elwell🇺🇸 · H. B. Tran Tan🇺🇸 · U. C. Perera🇺🇸 · H. W. T. Morgan🇺🇸 · A. N. Alexandrova🇺🇸 · Andrei Derevianko🇺🇸 · Eric R. Hudson🇺🇸
The population dynamics of the 229Th isomeric state is studied in a solid-state host under laser illumination. A photoquenching process is observed, where off-resonant vacuum-ultraviolet (VUV) radiation leads to relaxation of the isomeric state. The cross-section for this photoquenching process is measured and a model for the decay process, where photoexcitation of electronic states within the material bandgap opens an internal conversion decay channel, is presented and appears to reproduce the measured cross-section.