High-precision mass measurement of doubly magic Pb
Kathrin Kromer🇩🇪 · Chunhai Lyu🇩🇪 · Menno Door🇩🇪 · Pavel Filianin🇩🇪 · Zoltán Harman🇩🇪 · Jost Herkenhoff🇩🇪 · Wenjia Huang🇫🇷 · Christoph H. Keitel🇩🇪 · Daniel Lange🇩🇪 · Yuri N. Novikov🇷🇺 · Christoph Schweiger🇩🇪 · Sergey Eliseev🇩🇪 · Klaus Blaum🇩🇪
The absolute atomic mass of Pb has been determined with a fractional uncertainty of by measuring the cyclotron-frequency ratio of Pb to Xe with the high-precision Penning-trap mass spectrometer Pentatrap and computing the binding energies and of the missing 41 and 26 atomic electrons, respectively, with the ab initio fully relativistic multi-configuration Dirac-Hartree-Fock (MCDHF) method. has been measured with a relative precision of . and have been computed with an uncertainty of 9.1 eV and 2.1 eV, respectively, yielding u (u eV/c) for the Pb neutral atomic mass. This result agrees within with that from the Atomic-Mass Evaluation (AME) 2020, while improving the precision by almost two orders of magnitude. The new mass value directly improves the mass precision of 14 nuclides in the region of Z=81-84 and is the most precise mass value with A>200. Thus, the measurement establishes a new region of reference mass values which can be used e.g. for precision mass determination of transuranium nuclides, including the superheavies.