Measurement of the Zn,Ti(n,p) Cross Sections using a DD Neutron Generator for Medical Isotope Studies
Andrew Voyles · M.S. Basunia · Jon Batchelder🇺🇸 · Joseph Bauer · Tim Becker · Lee Bernstein🇺🇸 · Eric Matthews · Paul Renne · Daniel Rutte · Mauricio Unzueta · Karl van Bibber🇺🇸
Cross sections for the Ti(n,p)Sc and Zn(n,p)Cu reactions have been measured for quasi-monoenergetic DD neutrons produced by the UC Berkeley High Flux Neutron Generator (HFNG). The HFNG is a compact neutron generator designed as a "flux-trap" that maximizes the probability that a neutron will interact with a sample loaded into a specific, central location. The study was motivated by interest in the production of Sc and Cu as emerging medical isotopes. The cross sections were measured in ratio to the In(n,n')In and In(n,n')In inelastic scattering reactions on co-irradiated indium samples. Post-irradiation counting using an HPGe and LEPS detectors allowed for cross section determination to within 5% uncertainty. The Zn(n,p)Cu cross section for 2.76 MeV neutrons is reported as 49.3 2.6 mb (relative to In) or 46.4 1.7 mb (relative to In), and the Ti(n,p)Sc cross section is reported as 26.26 0.82 mb. The measured cross sections are found to be in good agreement with existing measured values but with lower uncertainty (< 5%), and also in agreement with theoretical values. This work highlights the utility of compact, flux-trap DD-based neutron sources for nuclear data measurements and potentially the production of radionuclides for medical applications.